Technical Annual Status Report (Stage 2) for the CLRTAP Inventory Review: Synthesis and Assessment Country report

TIME SERIES

Party: MK Submission year: 2025

The aim of this test is to identify instances of dips, jumps, and sudden changes in time series data reported by countries. The analysis was limited to data provided in NFR02, NFR09, NFR14 and NFR19 reporting format. Only data reported for at least three years were considered. Years where only NFR02 or NFR09 sectors were available have been converted to NFR14/NFR19. Only the converted sectors are in the time series analysis.

The table below shows data, where outliers in the time series were identified based on the following methodology: Reported time series data were log 10-transformed prior to analysis to reduce intra-series variability and improve general time series linearity. A linear regression was subsequently applied to the log-transformed values for each time series.

An individual value within the time series was identified as a dip/jump if the respective residual value (regression forecast value - reported value) is more than 2 standard deviations from the mean of all residuals in the time series. Only time series where the flagged data value contributed a significant fraction (>3%) of the national total for the given year are included in this dataset for expert review.

Time series where sigma grow largely (i.e. more than 20% of the time series mean value) because of extreme variation in the emission data are also flagged. Zero values indicate small numbers rounded to zero.

The test was performed for the following time series (if data was available):
Main pollutants: 1990 – 2023
HMs and POPs: 1990 - 2023
PMs: 2000 - 2023

If there is a number and a notation key reported, the difference is the number.

Color Key
	Indicates a dip in the time series data
	Indicates a jump in the time series data
	Indicates time series data with large sigma

MAIN (Unit = Mg)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
NOx	1A2a	1834	977	1250	1002	490	700	17	139	1814	1321	1269	791	861	1195	1196	2070	2638	3399	2919	2054	2753	2020	3009	2698	2019	1522	1356	926	1089	1418	1344	1281	776	555
NOx	1A4ai	143	25	42	26	26	26	26	26	899	1183	392	221	2891	1113	813	1643	1324	1250	711	1196	1137	489	605	581	520	617	664	603	543	525	422	338	55	40
NMVOC	1A2a	202	219	258	207	101	203	1	29	504	341	246	208	171	312	348	579	684	873	763	425	641	549	778	660	549	439	412	268	349	501	529	494	309	176
NMVOC	1A2gviii	105	106	102	99	91	82	181	144	160	128	157	154	162	188	206	714	170	194	201	138	135	146	145	134	142	171	298	296	295	286	145	205	163	179
NMVOC	1A3biv	998	1058	1590	1740	841	1335	1566	1992	2066	2031	2160	441	670	628	800	13	14	14	10	12	56	56	53	46	17	22	27	30	22	15	6	12	31	24
NMVOC	1A4bi	5630	4940	5383	6017	5749	5746	5742	5738	5451	5740	6783	5275	5239	5823	5815	5205	5168	4833	4817	4816	4744	5166	5596	5486	5717	5481	4591	5228	4336	4453	4594	4627	4456	4127
NMVOC	1B2av	2665	2058	1252	2687	528	3728	1506	2067	2180	2314	1775	4316	801	1523	1726	1811	1843	2046	2053	2013	2324	2550	2576	2819	2692	2972	3356	3872	3925	4243	3745	4166	4607	4746
NMVOC	2D3a	2434	2441	2467	2479	2349	2370	2390	2403	2415	2426	2437	2446	2428	2436	2442	1099	1549	1878	1843	1467	2320	2176	2178	2154	2301	2449	2497	2627	2667	2787	2857	2623	2403	2605
NMVOC	2D3d	3779	3446	3232	3033	2753	2562	2707	2766	2829	2739	2804	2809	2797	2851	2762	1517	2541	2666	2752	2300	2594	2848	3425	3315	3205	3309	3091	2683	2522	2627	2487	2634	2578	2796
NMVOC	3B1b	1041	1021	1032	999	1003	1012	1040	999	912	902	870	861	828	889	853	833	845	830	803	892	880	803	799	686	718	808	810	828	792	667	716	497	403	497
NMVOC	3De	1135	1114	1125	1117	1116	1109	1110	1105	1112	1104	1063	1070	1132	1121	1088	1057	1054	926	915	872	964	963	1065	1084	1086	1087	1090	1089	1087	1088	1085	1084	1081	1076
NMVOC	NATIONALTOTAL	40829	35773	37340	39792	33919	38733	36784	38032	38700	38881	39842	34493	31532	31081	31419	23245	24477	25157	24980	23048	24313	24927	25000	24479	24251	23538	23398	23934	23245	22920	21719	21807	22151	21255
NMVOC	NTCOMPL(NECD)	40829	35773	37340	39792	33919	38733	36784	38032	38700	38881	39842	34493	31532	31081	31419	18648	24477	25157	24980	23048	24313	24927	25000	24479	24251	23538	23398	23934	23245	22920	17847	18319	18709	18126
NMVOC	NTCOMPLIANCE	40829	35773	37340	39792	33919	38733	36784	38032	38700	38881	39842	34493	31532	31081	31419	23245	24477	25157	24980	23048	24313	24927	25000	24479	24251	23538	23398	23934	23245	22920	21719	21807	22151	21255
SOx	1A1a	102149	81794	78885	81346	83802	88839	85118	88368	96981	88482	97887	100995	88937	87246	87637	86823	84412	87735	67354	97049	77477	96048	82925	75027	76901	69507	56267	49188	53855	108035	88868	83137	91863	102187
SOx	1A2a	1402	1976	2282	1828	894	1921	2	254	4734	3165	2136	1758	1292	2651	3020	4866	5810	7674	6778	3506	5410	4968	6863	5881	4964	3997	3729	2308	2809	4369	3401	3562	2007	1290
SOx	NATIONALTOTAL	112403	91443	88657	91133	90275	96527	90541	94839	109368	99310	106257	108281	96122	94714	95641	94769	93179	98522	76877	103098	85688	103453	91344	82063	82709	75032	63293	54744	59821	115445	93453	88612	94945	105122
SOx	NTCOMPL(NECD)	112403	91443	88657	91133	90275	96527	90541	94839	109368	99310	106257	108281	96122	94714	95641	94769	93179	98522	76877	103098	85688	103453	91344	82063	82709	75032	63293	54744	59821	115445	93453	88612	94945	105122
SOx	NTCOMPLIANCE	112403	91443	88657	91133	90275	96527	90541	94839	109368	99310	106257	108281	96122	94714	95641	94769	93179	98522	76877	103098	85688	103453	91344	82063	82709	75032	63293	54744	59821	115445	93453	88612	94945	105122
NH3	11B											96	105	110	38	36	62	72	689	301	21	94	174	386	57	23	63	43	268	56	314	25	246	39	115
NH3	1B2d									456	375	382	566	317	322	288	243	245	261	242	297	297	299	258	207	178	164	160	148	146	136	130	129	122	117
NH3	3B1b	949	931	941	911	914	922	948	911	831	823	794	785	755	811	778	759	770	757	732	813	803	732	729	625	655	737	738	755	722	608	653	453	368	453
NH3	3B3	873	853	865	977	923	924	985	994	1016	1145	1029	951	1009	975	816	812	882	1344	1237	973	962	949	872	855	818	907	1003	982	932	652	769	868	864	906
CO	1A1a	2657	2096	2021	2085	2147	2277	2181	2264	2503	2284	2536	2614	2304	2249	2248	2227	2171	2283	1019	1803	1748	2512	3354	1982	2034	1908	1684	1763	1030	1803	1095	807	1031	1179
CO	1A2a	1504	2064	2388	1913	936	1999	2	265	4928	3299	2240	1855	1382	2796	3178	5155	6139	8060	7106	3705	5714	5197	7211	6159	5193	4180	3903	2431	3007	4616	3843	3917	2257	1403
CO	1A3biii	2736	3758	4450	4641	4024	4512	4472	4574	4634	4619	4793	3928	4238	1	3510	576	540	588	542	545	434	383	324	323	1628	1759	1822	1777	1632	1577	1353	1358	1688	1648
CO	1A4bi	38327	34044	37009	41252	39434	39390	39346	39302	37228	39322	46251	35968	35845	39781	39782	35476	35132	32883	32673	32613	32148	34953	37820	37778	36986	38572	37021	31043	29345	30149	31122	31386	30229	28037
CO	NATIONALTOTAL	106657	89626	99348	105443	94557	100054	96614	99793	103995	105169	112876	89010	91108	89260	94012	74125	69772	70771	66081	62193	61331	62942	65340	62927	60673	61500	61470	53735	53006	53566	48821	50071	46613	44179
CO	NTCOMPL(NECD)	106657	89626	99348	105443	94557	100054	96614	99793	103995	105169	112876	89010	91108	89260	94012	74125	69772	70771	66081	62193	61331	62942	65340	62927	60673	61500	61470	53735	53006	53566	48821	50071	46613	44179
CO	NTCOMPLIANCE	106657	89626	99348	105443	94557	100054	96614	99793	103995	105169	112876	89010	91108	89260	94012	74125	69772	70771	66081	62193	61331	62942	65340	62927	60673	61500	61470	53735	53006	53566	48821	50071	46613	44179

PM (Unit = Mg)

		2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
PM2.5	11B	4933	612	171	76	30	7	90	4281	247	11	14	386	708	106	133	225	122	575	40	665	56	3396	86	131
PM2.5	2C2	10112	1517	2607	11627	14370	12333	10229	5997	7451	1355	5254	9783	8988	11494	5999	3965	2592	21	31	47	50	44	23	7
PM10	11B	6029	748	209	93	37	9	110	5232	302	13	17	472	865	129	162	275	149	703	49	813	69	4150	106	160
PM10	2A5a	246	174	143	37	17	141	230	348	355	289	342	355	352	389	361	379	416	392	393	419	389	366	343	381
PM10	2C2	14326	2149	3693	16471	20358	17472	14491	8496	10555	1919	7443	13859	12733	16111	8451	5563	3672	29	44	67	70	63	33	10
PM10	2D3b	984	412	359	373	448	542	393	305	510	696	860	690	778	952	1116	12	10	14	16	16	17	17	16	17
PM10	3Dc	1928	1941	2053	2033	1973	1917	1911	1680	1660	1582	1749	1747	1931	1966	1971	1972	1977	1975	1972	1973	1968	1966	1961	1951
TSP	11B	9317	1155	323	144	57	14	170	8085	467	20	27	730	1337	200	251	425	230	1086	76	1256	107	6414	163	248
TSP	2A5a	502	356	291	75	35	288	470	709	724	590	698	725	718	794	736	773	848	799	802	855	794	746	699	777
TSP	2C2	16854	2528	4344	19378	23950	20555	17049	9995	12418	2258	8756	16304	14980	18954	9942	6524	4320	35	52	79	83	74	39	12
TSP	3Dc	1928	1941	2053	2033	1973	1917	1911	1680	1660	1582	1749	1747	1931	1966	1971	1972	1977	1975	1972	1973	1968	1966	1961	1951
BC	11B	444	55	15	7	3	1	8	385	22	1	1	35	64	10	12	20	11	52	4	60	5	306	8	12
BC	1A2gviii	35	37	39	40	28	105	43	58	58	39	41	44	44	42	44	35	32	32	34	37	41	43	45	42
BC	1A4ai	48	7	95	50	41	63	58	55	41	65	59	25	35	27	28	27	29	27	25	24	21	21	12	6
BC	2C2	1011	152	261	1163	1437	1233	1023	600	745	135	525	978	899	1149	600	387	259	2	3	5	5	4	2	1

HM (Unit = g)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
Pb	1A1a	886861	698921	677444	695471	723704	762979	729038	755477	839771	763404	808791	863143	750280	749606	752756	744492	700787	715496	794746	766962	706416	803194	765509	657006	669989	604567	498748	432566	475308	566897	435987	358343	464860	483650
Pb	1A2a	187302	285947	328576	263245	128740	281473	3	36508	692389	461500	306336	256302	184788	386375	442356	712462	847346	1118350	988458	504211	784469	725810	1001068	854928	725227	585537	547220	338003	414327	645908	511099	531996	301146	190370
Pb	1A2gviii	65077	62522	55683	57257	55222	55814	45394	128032	125564	113199	147197	158392	165517	205601	292505	168600	118908	125749	116535	73286	78623	84453	81759	78060	69286	181600	430908	426559	416557	385908	117498	222117	110139	160467
Pb	1A3bi	89093506	68602775	76903399	72319879	72319879	78564788	78046806	79470776	79326235	79651039	82324210	81595190	86890465	82384938	17134064	231	217	242	244	260	272	297	268	300	199	205	223	223	227	236	175	208	226	248
Pb	1A4bi	280371	268395	287261	314746	301325	299876	298428	296980	275768	297162	339189	262913	267906	294565	296900	257693	250049	234796	228466	225115	222806	239949	260502	260341	254327	265611	256025	216232	205923	212472	220262	222909	214137	199402
Pb	2C1	4071069	3475916	2522925	1627581	644207	383672	589338	1059260	1600092	1092081	2014496	2683543	4416819	3498475	3833309	3715797	4164251	4520190	3525026	3245608	3495650	3969004	2594648	1673880	2292911	2147496	259670	416398	408622	370526	277995	482180	380202	455968
Pb	2C5	131064150	116827700	139556800	130446050	124682350	134043050	141176050	155643000	169193300	118543300	102242667	81401978	72067200	39720600	20827800	197200	266800	104400	121800	226200						2913	4919	8235	11634	12058	11373	11373	12922	61645
Pb	2G	3419809	2584849	3031729	2714209	2217153	2199121	2175601	2576225	2535457	2429617	1955297	1880817	1770273	2054081	1921585	1859648	1978816	1880032	1438640	1433152	2333185	3457441	3311616	2026640	3019969	3284960	2341808	2572304	2706369	3346112	3853360	4016432	4685968	4758096
Pb	NATIONALTOTAL	236187514	199294497	230346140	214952452	205689789	224032770	231367689	246832568	261892002	210220396	196926319	173756330	172008980	133474647	47036799	7916461	8569570	8961127	7448009	6736435	7888622	9534633	8276351	5837291	7322716	7399825	4699895	4783412	5000526	5931986	5770271	6219439	6562346	6691607
Pb	NTCOMPL(NECD)	236187514	199294497	230346140	214952452	205689789	224032770	231367689	246832568	261892002	210220396	196926319	173756330	172008980	133474647	47036799	7916461	8569570	8961127	7448009	6736435	7888622	9534633	8276351	5837291	7322716	7399825	4699895	4783412	5000526	5931986	5770271	6219439	6562346	6691607
Pb	NTCOMPLIANCE	236187514	199294497	230346140	214952452	205689789	224032770	231367689	246832568	261892002	210220396	196926319	173756330	172008980	133474647	47036799	7916461	8569570	8961127	7448009	6736435	7888622	9534633	8276351	5837291	7322716	7399825	4699895	4783412	5000526	5931986	5770271	6219439	6562346	6691607
Cd	1A2a	2531	3847	4422	3542	1732	3784	0	491	9313	6213	4123	3448	2488	5230	5976	10627	12276	15442	13409	6799	11218	9803	14324	11550	9795	7923	7387	4564	6849	9891	13229	11420	7309	3344
Cd	1A2gviii	5017	4806	4252	4387	4106	4042	4125	5757	4849	5252	6937	7373	7559	7288	8606	33057	9228	9183	9573	5790	6276	7064	6855	5986	5837	6810	11510	11454	11401	10910	7413	9023	7422	7939
Cd	1A4bi	121897	105857	115619	129530	123746	123727	123708	123688	117800	123722	146789	114177	113067	125832	125539	112745	112262	104946	104861	104994	103407	112722	122491	122489	120471	126081	121429	102261	97707	100940	104756	106071	102736	95663
Cd	2C5	350738	316125	372403	347075	330930	356556	377167	415096	449619	317739	272250	218352	194210	110555	53865	510	690	270	315	585						132	224	374	529	548	517	517	587	2802
Cd	2C6	892075	883945	772050	375680	368540	1428815	1622145	407525	595115	407100	260000	260000	280000	140000	125000
Cd	NATIONALTOTAL	1528107	1439602	1384583	978198	934947	2026611	2236579	1066590	1317807	990442	835607	745507	730747	521293	453727	288524	264756	264412	264771	253161	250813	269587	272397	246385	249460	246725	243082	226961	227687	243002	224569	235347	234978	230177
Cd	NTCOMPL(NECD)	1528107	1439602	1384583	978198	934947	2026611	2236579	1066590	1317807	990442	835607	745507	730747	521293	453727	288524	264756	264412	264771	253161	250813	269587	272397	246385	249460	246725	243082	226961	227687	243002	224569	235347	234978	230177
Cd	NTCOMPLIANCE	1528107	1439602	1384583	978198	934947	2026611	2236579	1066590	1317807	990442	835607	745507	730747	521293	453727	288524	264756	264412	264771	253161	250813	269587	272397	246385	249460	246725	243082	226961	227687	243002	224569	235347	234978	230177
Hg	1A2a	11400	16995	19557	15668	7663	16670	4	2173	41026	27370	18270	15640	11536	23518	26858	42914	50991	67105	59317	30637	47173	43424	59649	51151	43390	35032	32857	20571	24965	38588	30202	31639	18073	11712
Hg	2C1	88502	75563	54846	35382	14004	8341	12812	23027	34785	23741	43793	58338	96018	76054	83333	80778	90527	98265	76631	70557	75992	86283	56405	36389	49846	46685	13157	21098	20704	18773	14085	24430	19264	23102
Hg	2K	19573	19748	19914	20023	19573	19748	19914	20023	20127	20216	20311	20387	20237	20299	20352	20385	20419	20452	20486	20527	20573	20598	20623	20658	20692	20713	20737	20753	20771	20763	20688	18377	18300	18262

POP (Unit = mg)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
DIOX	1A2a	288	435	500	400	196	427	0	56	1051	701	466	390	282	588	672	1088	1292	1701	1502	768	1196	1103	1525	1300	1102	889	831	514	635	986	806	828	473	293
DIOX	1A2b	467	371	372	373	343	313	0	187	374	357	416	390	254	121	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0	0
HCB	1A2a	865	1323	1520	1218	595	1302		169	3204	2137	1417	1186	855	1800	2057	3699	4259	5327	4617	2337	3884	3374	4962	3974	3371	2728	2543	1571	2410	3455	4817	4108	2651	1183
HCB	1A4bi	46856	40664	44420	49772	47549	47543	47537	47531	45276	47544	56422	43887	43453	48362	48247	43339	43159	40344	40318	40373	39761	43346	47103	47103	46329	48487	46698	39325	37575	38819	40287	40792	39512	36792
PCB	2C5	124257100	126130200	127625200	114811700	106169100	117581300	131060900	141312400	146487800	114625000	90937333	79439022	74288800	56442400	11491200	108800	147200	57600	67200	124800						6884800	11627200	19463600	27497600	28501200	26881400	26881400	30542200	145706600
PCB	2K	202800000	203396400	205600000	206600000	195726500	197480000	199139800	200234000	201270500	202157800	203111200	203865100	202365400	202989200	203519600	203851400	204194100	204517700	204861900	205272200	205728400	205979400	206229400	206576900	206917200	207127800	207370200	207530100	207713200	207713200	208713200	209713200	210713200	211713200