Technical Annual Status Report (Stage 2) for the CLRTAP Inventory Review: Synthesis and Assessment Country report

TIME SERIES

Party: GR Submission year: 2025

The aim of this test is to identify instances of dips, jumps, and sudden changes in time series data reported by countries. The analysis was limited to data provided in NFR02, NFR09, NFR14 and NFR19 reporting format. Only data reported for at least three years were considered. Years where only NFR02 or NFR09 sectors were available have been converted to NFR14/NFR19. Only the converted sectors are in the time series analysis.

The table below shows data, where outliers in the time series were identified based on the following methodology: Reported time series data were log 10-transformed prior to analysis to reduce intra-series variability and improve general time series linearity. A linear regression was subsequently applied to the log-transformed values for each time series.

An individual value within the time series was identified as a dip/jump if the respective residual value (regression forecast value - reported value) is more than 2 standard deviations from the mean of all residuals in the time series. Only time series where the flagged data value contributed a significant fraction (>3%) of the national total for the given year are included in this dataset for expert review.

Time series where sigma grow largely (i.e. more than 20% of the time series mean value) because of extreme variation in the emission data are also flagged. Zero values indicate small numbers rounded to zero.

The test was performed for the following time series (if data was available):
Main pollutants: 1990 – 2023
HMs and POPs: 1990 - 2023
PMs: 2000 - 2023

If there is a number and a notation key reported, the difference is the number.

Color Key
	Indicates a dip in the time series data
	Indicates a jump in the time series data
	Indicates time series data with large sigma

MAIN (Unit = Mg)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
NOx	11B	774	293	849	885	773	507	209	612	1918	122	2362	250	24	36	93	79	235	3095	482	525	222	95	351	27	17	69	200	89	66	1626	137	2117	828	7025
NOx	1A2gviii	17867	17174	17126	15120	14992	18370	17859	17855	15049	10475	11893	12831	10067	6765	4240	14586	16277	16164	13860	10026	8073	6807	8110	4019	4305	4606	5100	5256	5346	4240	3871	3390	5346	2567
NOx	1A3ai(ii)	9476	8788	10348	10481	10964	10390	9887	10448	10634	11522	11657	10892	10154	10431	10839	10571	11384	12186	12234	11467	10818	11260	9939	10368	11937	11552	12419	14137	15426	16294	5148	9320	14909	16123
NOx	1A3bii	22591	23516	22707	22591	22367	19781	19449	19209	18952	18641	17796	17325	16736	16252	15970	15020	14856	14858	14961	12875	11470	9340	7909	8724	10454	10203	10022	9888	11868	13023	12951	12452	13088	12579
NOx	1A3dii	40636	41738	42746	39159	41155	39096	33463	40533	62590	60778	34237	46966	39746	36816	40197	45310	38800	35542	31306	51061	40369	32351	34902	28341	29299	34724	36026	36869	39822	41244	35246	36455	39030	40158
NMVOC	11B	2322	880	2548	2656	2319	1522	628	1837	5755	366	7085	749	71	107	280	236	704	9285	1445	1574	667	285	1054	80	52	208	601	268	197	4877	411	6351	2484	21076
NMVOC	1A3bii	29424	30492	29098	28771	28260	25285	24595	23841	23019	22075	19155	18125	18340	17950	16893	15728	13875	12910	12580	11253	9245	7154	6045	6042	7291	7220	6949	5602	7053	7843	7599	6300	6270	6048
NMVOC	1A3bv	32854	32515	31109	29572	29311	28623	26915	26457	25974	23584	20355	19912	19450	20640	19760	17707	14597	13842	12445	13934	14385	13878	16137	15705	15562	14709	14112	13633	10928	10846	9383	9678	9675	9619
NMVOC	1A3di(i)	4338	3982	4577	5338	5672	6101	5364	5379	5999	5330	6152	6364	5755	5893	5945	9824	10651	5827	5700	4843	5046	4947	4048	3819	3352	3233	3120	3867	3954	4561	2908	3304	3594	3682
NMVOC	1A4bi	18058	18233	18220	18213	18202	18164	18227	18293	18165	17947	17989	17973	17761	17728	17773	17715	17445	18542	14923	12926	10875	14663	17329	15282	15136	15713	13548	13963	12782	12409	11534	12830	13041	14164
NMVOC	1A4cii	9038	9452	8979	8910	8931	8731	8769	8766	8766	8766	8766	8677	9075	7500	6762	6578	6452	6265	6068	5543	4941	2997	12957	3513	1368	1402	1085	1998	973	1307	1942	1297	2256	1476
SOx	11B	155	59	170	177	155	101	42	122	384	24	472	50	5	7	19	16	47	619	96	105	44	19	70	5	3	14	40	18	13	325	27	423	166	1405
NH3	3B2	3561	3574	3563	3580	3619	3647	3658	3653	3672	3681	3697	3753	3725	3702	3630	3615	3631	3658	3655	3672	3661	3665	3610	3541	3487	3596	3569	3571	3663	3667	3672	3722	3708	3693
NH3	3B4h	4526	4538	4531	4531	4527	4480	4573	4502	4620	4483	4535	4493	4321	4146	4146	3976	3765	3620	3587	3512	3475	3580	3559	3450	2709	2640	2623	2533	2379	2281	1604	1604	1310	1604
NH3	3Da1	29596	28480	27223	21429	19964	22058	22546	21429	21499	20452	18847	18149	17660	17241	17800	15636	14659	15847	14561	10854	14474	12366	11423	12752	11205	12109	12692	12644	11806	12271	12950	14216	11157	11788
NH3	NATIONALTOTAL	95712	93252	90949	85343	81311	85084	86181	85322	85368	84757	82090	81129	80369	79795	82423	80023	77562	78367	74747	70388	75744	74656	72540	72290	68711	67532	67538	67048	66489	66375	68570	68081	64484	66227
NH3	NTCOMPL(NECD)	95712	93252	90949	85343	81311	85084	86181	85322	85368	84757	82090	81129	80369	79795	82423	80023	77562	78367	74747	70388	75744	74656	72540	72290	68711	67532	67538	67048	66489	66375	68570	68081	64484	66227
NH3	NTCOMPLIANCE	95712	93252	90949	85343	81311	85084	86181	85322	85368	84757	82090	81129	80369	79795	82423	80023	77562	78367	74747	70388	75744	74656	72540	72290	68711	67532	67538	67048	66489	66375	68570	68081	64484	66227
CO	1A3bii	213039	220769	212507	211277	208244	180832	176261	171735	166665	160713	146061	139117	131556	124938	118894	107175	109847	100538	98256	86270	72457	55666	46840	44675	57034	53801	51676	45156	56709	63102	58662	49627	49252	47297
CO	1A4bi	125470	127153	126975	126882	126792	126587	128356	129183	128140	126041	126837	127088	125288	126052	126134	125683	125028	133493	110013	96442	83511	113117	134028	117846	118474	125460	108025	110761	103069	102068	95345	105141	107439	115437
CO	1A4cii	44117	46049	43924	43701	43768	43123	43245	43234	43234	43234	43234	42650	44235	34680	31698	30629	29598	29304	28356	26656	23774	12503	72740	19098	6807	6916	5296	10477	4619	6578	9561	6260	11680	7462
CO	1A5b																20579	25541	21547	27416	9833	9549	8488	8306	9265	7426	8125	7954	7285	4922	5357	11824	1425	11948	14229
CO	2C3	18000	18256	18404	18166	17893	16295	17803	16840	18675	20511	21776	21429	21815	22317	22418	22044	22413	22783	22397	18728	19147	23616	23437	24236	24949	26099	26273	26336	26796	26491	27410	26647	27035	26895
CO	3F	30816	31712	29893	29553	29256	27996	28544	28494	28114	27465	28225	27942	28394	28353	28522	27910	27020	26203	27651	29105	25709	25017	25159	24730	22976	20261	20363	21515	19360	18873	18378	18245	18046	18213

PM (Unit = Mg)

		2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
PM2.5	11B	2150	227	22	32	85	72	214	2818	439	478	203	87	320	24	16	63	182	81	60	1480	125	1927	754	6398
PM2.5	1A3dii	1372	1799	1532	1425	1671	1507	1657	1591	1354	2573	1948	1658	2015	1588	1628	1935	1963	2005	2174	2214	2117	1939	2033	2065
PM2.5	1A4bi	23454	23452	23283	23284	23312	23267	22860	24207	19400	16765	14271	19120	22572	19729	19408	20054	17315	17838	16304	15757	14672	16267	16563	17936
PM2.5	2A5b	3509	3617	3800	3321	3653	2736	3270	2772	3999	3168	2311	1019	718	921	1279	1341	1691	1340	952	1133	1289	1158	1329	1609
PM10	11B	2628	278	26	40	104	88	261	3444	536	584	248	106	391	30	19	77	223	99	73	1809	153	2356	921	7820
PM10	1A3dii	1509	1971	1673	1561	1835	1650	1814	1745	1481	2847	2149	1850	2251	1775	1818	2159	2192	2239	2428	2472	2365	2165	2268	2304
PM10	1A4bi	24043	24041	23869	23870	23898	23853	23435	24817	19888	17186	14622	19593	23132	20222	19894	20555	17748	18284	16711	16150	15037	16673	16975	18386
PM10	2A5b	35090	36166	38002	33214	36533	27357	32700	27717	39995	31680	23109	10193	7182	9214	12791	13410	16910	13402	9523	11325	12888	11583	13289	16090
TSP	11B	4062	429	41	61	161	135	404	5323	829	902	383	164	604	46	30	119	344	154	113	2796	236	3641	1424	12085
TSP	1A4bi	25242	25238	25049	25046	25078	25027	24588	26040	20869	18033	15338	20554	24265	21217	20875	21570	18623	19187	17534	16944	15775	17494	17810	19293
TSP	2A5b	117452	121052	127192	111152	122274	91547	109441	92765	133873	106039	77348	34115	24037	30841	42817	44888	56607	44863	31875	37909	43140	38770	44482	53856
BC	11B	194	20	2	3	8	6	19	254	39	43	18	8	29	2	1	6	16	7	5	133	11	173	68	576
BC	1A2e	463	448	477	425	402	428	397	398	456	413	400	397	319	211	256	314	245	256	264	249	277	210	217	236
BC	1A3ai(ii)	76	71	66	68	71	69	73	77	79	77	73	1572	68	69	80	72	77	83	100	101	38	76	116	118
BC	1A3aii(ii)	5	4	4	4	5	4	4	5	5	7	7	457	6	5	6	6	6	6	7	7	3	6	8	8
BC	1A3biii	1162	1213	1259	1309	1353	1395	1442	1477	1507	1517	1126	968	936	936	844	1472	870	870	814	805	679	622	667	603
BC	1A4bi	1939	1939	1929	1930	1931	1928	1918	2057	1668	1461	1276	1729	2074	1833	1825	1912	1651	1699	1579	1547	1442	1596	1627	1760
BC	1A4cii	824	835	921	1005	850	854	895	796	774	610	542	577	72	101	121	132	109	107	114	105	185	139	140	115

HM (Unit = g)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
Pb	1A1a	47249247	45121559	48392094	48115089	50659485	48380693	47082967	51700022	54307894	53321620	56661516	57916292	56877970	57566955	59588114	59578007	54682185	57150212	55348793	54881875	24582242	24955204	22247686	19699497	21869119	5244445	4766382	6136580	4557207	2415563	1065632	981067	869825	671074
Pb	1A2f	4766590	5116470	4783541	4748211	4629262	4637049	4272047	4109437	4314436	3519410	3821892	3975559	2901140	2314487	2296548	1666834	1378711	2146243	1477020	547036	1025969	475267	369627	343810	387002	333842	260881	355550	863716	685668	764444	955110	569315	575856
Pb	1A3bi	315783372	296429850	275932861	261369968	250472475	245339632	246605893	238881758	233719838	217529960	201796898	878226	922285	974134	1005032	4944	5112	5335	5152	5309	4736	4480	3676	3419	3176	3259	3288	3193	3020	2959	2441	2949	3042	3059
Pb	1A3bii	120835791	116068935	107464859	98836996	94977821	89555216	86089465	81094168	77163816	68448333	60967551	374328	381852	391019	383028	883	883	931	908	853	854	730	599	681	782	997	1016	702	841	929	898	912	942	920
Pb	1A3biv	12794239	13053873	10446199	12505784	13279397	13400010	13322238	12908564	13326929	13151625	12945369	93926	103619	108712	109052	417	381	378	401	408	481	487	493	489	447	404	400	378	387	383	319	365	371	363
Pb	1A3di(i)	437640	399100	454770	533260	564390	600960	532700	534570	602180	533140	619140	607500	543690	560870	566980	507480	548720	562250	550770	465960	484640	496080	405840	380690	331860	315230	303330	379742	390395	449390	284083	316332	337061	347365
Pb	1A4bi	916788	963813	960681	958804	955692	944866	957831	974877	935187	881315	891339	885726	827889	815113	827869	811120	802893	866593	726557	631367	656152	867389	1030565	881121	864065	918005	794361	810650	763989	740416	694581	749561	786486	822655
Pb	2G	13657	23697	23697	47966	103247	26578	24069	21638	7605	9957	33006	76675	117051	70482	111093	122226	132888	103606	99646	130301	90395	70560	40925	147039	172441	132182	162915	161818	218030	271656	174402	100162	307733	440138
Cd	1A1a	5713280	5461509	5853282	5821079	6125439	5855755	5699370	6251880	6563489	6446727	6850952	6997930	6872551	6959867	7196886	7200221	6613852	6911413	6698156	6628908	2986239	3028808	2704844	2395289	2689536	699043	636486	802609	630771	397401	216230	207860	197400	168721
Cd	1A2e	1148	933	1021	955	994	614	88021	88878	88140	89859	108911	106489	114370	95717	99872	117259	104649	106064	128562	119399	117639	119707	88852	48339	59927	80100	56492	59273	61952	57590	68527	45533	47294	54047
Cd	1A3di(i)	46360	42060	47610	56060	59150	62480	55740	55970	63540	56100	65460	64780	57970	60110	60900	54680	59200	60850	59690	465960	52320	53760	43920	41050	35700	33670	32330	40683	41942	48230	30044	33443	35276	36470
Cd	1A4bi	383584	384127	384090	384068	384032	383910	384080	384280	384244	383203	383325	383267	382604	382475	382617	382426	382326	412271	334407	294266	306915	405709	494802	421806	408428	427220	371001	378738	358435	346402	326306	352396	366150	385810
Cd	2G	585861	597836	610036	622530	654959	693212	1262356	1284824	1307269	1776014	239903	838705	558253	466542	448899	365626	344034	165503	315594	511305	449266	142733	263925	97428	104632	148057	142001	88035	100462	149902	106649	124650	135828	187125
Cd	3F	406573	418386	394392	389908	385983	369362	376592	375937	370914	362355	372387	368644	374615	374069	376303	368226	356479	345704	364805	383996	339195	330058	331927	326268	303128	267317	268661	283857	255427	249000	242468	240710	238087	240296
Cd	NATIONALTOTAL	7519069	7305785	7674961	7649369	7987978	7750526	8187261	8768314	9108499	9433706	8353886	9105022	8701801	8663987	8897453	8871880	8267282	8423997	8300024	8389297	4644407	4459251	4318220	3739884	4023324	2092248	1967113	2085258	1899089	1687108	1452217	1520564	1454692	1450535
Cd	NTCOMPL(NECD)	7519069	7305785	7674961	7649369	7987978	7750526	8187261	8768314	9108499	9433706	8353886	9105022	8701801	8663987	8897453	8871880	8267282	8423997	8300024	8389297	4644407	4459251	4318220	3739884	4023324	2092248	1967113	2085258	1899089	1687108	1452217	1520564	1454692	1450535
Cd	NTCOMPLIANCE	7519069	7305785	7674961	7649369	7987978	7750526	8187261	8768314	9108499	9433706	8353886	9105022	8701801	8663987	8897453	8871880	8267282	8423997	8300024	8389297	4644407	4459251	4318220	3739884	4023324	2092248	1967113	2085258	1899089	1687108	1452217	1520564	1454692	1450535
Hg	1A1a	1708036	1635376	1750750	1741735	1831160	1753315	1706815	1869447	1962072	1930494	2053173	2094919	2057929	2086466	2154367	2157342	1985952	2077113	2025528	1993688	1886617	1915372	1915113	1696272	1053669	931405	710833	775810	852632	716509	324392	300722	297276	228104
Hg	3F	64682	66561	62744	62031	61406	58762	59912	59808	59009	57647	59243	58648	59598	59511	59866	58581	56713	54998	58037	61090	53963	52509	52806	51906	48225	42528	42741	45159	40636	39614	38574	38295	37878	38229
Hg	5C1biii	2090	2090	2090	2090	2090	2090	2090	2090	2090	2090	2090	2090	5712	10902	13584	25904	31350	42562	50188	172043	87967	77677	48006	52911	61721	70532	54020	48188	41251	35051	31578	34585	36507	43516
Hg	NATIONALTOTAL	2273426	2223002	2303247	2298334	2382416	2306072	2252147	2414684	2523836	2423937	2591570	2656519	2574667	2566281	2651594	2711971	2567543	2716061	2618396	2648207	2458703	2438046	2405252	2188037	1557412	1422605	1225815	1288083	1375600	1209276	808092	846849	739390	620980
Hg	NTCOMPL(NECD)	2273426	2223002	2303247	2298334	2382416	2306072	2252147	2414684	2523836	2423937	2591570	2656519	2574667	2566281	2651594	2711971	2567543	2716061	2618396	2648207	2458703	2438046	2405252	2188037	1557412	1422605	1225815	1288083	1375600	1209276	808092	846849	739390	620980
Hg	NTCOMPLIANCE	2273426	2223002	2303247	2298334	2382416	2306072	2252147	2414684	2523836	2423937	2591570	2656519	2574667	2566281	2651594	2711971	2567543	2716061	2618396	2648207	2458703	2438046	2405252	2188037	1557412	1422605	1225815	1288083	1375600	1209276	808092	846849	739390	620980

POP (Unit = mg)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022	2023
DIOX	1A4bi	24535	24827	24800	24786	24769	24721	24936	25063	24867	24505	24612	24624	24294	24341	24383	24296	23708	24889	19983	17145	14706	19484	22674	19492	19041	19619	17013	17562	15905	15240	14234	15685	16053	17231
HCB	1A4bi	147549	147773	147758	147749	147734	147683	147743	147824	147795	147378	147425	147398	147122	147060	147121	147041	147002	158525	128586	113149	118017	156011	190275	162218	157075	164302	142679	145655	137848	133218	125485	135523	140813	148380
HCB	5C1biii	18000	18000	18000	18000	18000	18000	18000	18000	18000	18000	18000	18000	49200	93900	117000	223119	270025	366600	432279	1481853	757679	669057	413491	455738	531623	607507	465291	415058	355309	301904	271985	297893	314447	374812