Technical Annual Status Report (Stage 2) for the CLRTAP Inventory Review: Synthesis and Assessment Country report

TIME SERIES

Party: FI Submission year: 2024

The aim of this test is to identify instances of dips, jumps, and sudden changes in time series data reported by countries. The analysis was limited to data provided in NFR02, NFR09, NFR14 and NFR19 reporting format. Only data reported for at least three years were considered. Years where only NFR02 or NFR09 sectors were available have been converted to NFR14/NFR19. Only the converted sectors are in the time series analysis.

The table below shows data, where outliers in the time series were identified based on the following methodology: Reported time series data were log 10-transformed prior to analysis to reduce intra-series variability and improve general time series linearity. A linear regression was subsequently applied to the log-transformed values for each time series.

An individual value within the time series was identified as a dip/jump if the respective residual value (regression forecast value - reported value) is more than 2 standard deviations from the mean of all residuals in the time series. Only time series where the flagged data value contributed a significant fraction (>3%) of the national total for the given year are included in this dataset for expert review.

Time series where sigma grow largely (i.e. more than 20% of the time series mean value) because of extreme variation in the emission data are also flagged. Zero values indicate small numbers rounded to zero.

The test was performed for the following time series (if data was available):
Main pollutants: 1990 – 2022
HMs and POPs: 1990 - 2022
PMs: 2000 - 2022

If there is a number and a notation key reported, the difference is the number.

Color Key
	Indicates a dip in the time series data
	Indicates a jump in the time series data
	Indicates time series data with large sigma

MAIN (Unit = Mg)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022
NOx	1A3ai(ii)	3549	3331	2914	2724	2878	3101	3334	3439	3478	3732	3588	3706	3702	3832	4402	4652	5134	6056	6712	6319	6308	7536	7379	7406	7420	7471	7961	7416	8331	9157	3321	3232	5986
NOx	1A3di(i)	49957	47636	59342	48698	39356	32303	35507	37977	40290	41788	47251	41105	46766	46310	36041	34664	37957	30472	25587	15512	13000	11699	6589	7027	5092	16605	15834	19502	17975	18608	17116	15647	18819
NOx	1A4bi	6553	6442	6470	6401	6302	5884	6168	6176	6339	6191	5760	6403	6379	6406	6401	6381	6154	6174	5842	6090	6741	5552	6005	5536	5545	5165	5552	5383	5217	5053	4601	5001	4444
NMVOC	1A4bi	18122	18241	18279	18330	19159	17143	18458	18561	19265	18788	16874	19287	19436	19946	20217	21189	20262	21147	20881	22011	24335	20867	22764	21433	21707	20475	22347	21971	21562	21240	17538	19656	18181
NMVOC	1B2aiv	6600	5400	6510	7231	6478	5000	4565	4745	4876	4913	4748	4590	4085	4379	3956	3196	3809	3892	3605	3411	4881	3493	3851	3778	3064	3035	3331	3048	2948	2705	2532	2234	1876
NMVOC	2D3a	3065	2972	2928	2929	3028	3191	3272	3451	3671	3823	4037	4215	4602	4478	4386	4763	4963	5256	5393	5744	5258	6082	5395	5572	5772	6143	6199	6450	6270	6330	12067	8093	6692
NMVOC	3Da2a	3981	3843	3836	3865	3670	3716	3767	3697	3546	3556	3511	3548	3526	3448	3402	3322	3215	3091	3014	3037	2951	2921	2970	3103	2711	2658	2523	2456	2339	2175	2175	2156	2101
SOx	2C1	2867	2766	857	789	785	763	880	947	774	779	770	732	750	982	1185	1135	1158	1196	1135	1017	1043	916	617	563	497	661	744	730	739	899	843	967	848
NH3	1A4bi	907	918	920	923	962	863	929	934	969	945	873	998	1007	1035	1050	1092	1044	1093	1095	1154	1290	1106	1207	1137	1151	1091	1188	1165	1144	1125	990	1109	1022
NH3	2C7c	0	0	0	0	0	0	0	0	0	2550	0	0	1	1	0	0	1	0	0	0	0	0	0	0	0	0	0	0	0	0	1	1	0
CO	1A2d	29503	25358	22448	26510	29017	28401	26653	28693	29128	29310	29413	26721	27149	26519	28823	23834	26426	23580	19631	14246	17883	17691	18124	19355	19511	17740	18278	19783	21878	20602	19605	17433	13452
CO	1A3dii	22554	23187	23289	23099	22934	23464	23330	23654	24095	24644	23473	23193	23347	22743	22598	22947	23764	24001	19831	19836	21110	16328	17480	18904	19479	19931	19123	19310	19577	19777	22634	25281	20958
CO	1A4bi	125262	126601	126874	127274	132693	119062	128127	128776	133619	130310	120315	137573	138725	142513	144546	150340	143780	150349	150527	158677	177393	151995	165882	156143	158075	149842	163083	159927	157061	154450	135818	152185	140223

PM (Unit = Mg)

		2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022
PM2.5	1A2d	3140	2460	2381	2999	3097	2447	2092	1913	1618	1125	1374	1345	1431	1300	1303	1399	1330	1410	1295	1019	990	870	734
PM10	1A2d	4416	3545	3289	3966	4107	3265	2927	2651	2223	1591	1907	1856	1971	1794	1793	2035	1832	1948	1841	1490	1438	1562	1204
PM10	1A5a	487	585	875	687	817	814	710	622	658	723	825	823	912	785	849	811	969	952	619	1302	1035	1564	1917
TSP	1A2d	4934	3945	3620	4292	4451	3558	3261	2958	2451	1774	2111	2058	2185	2039	2036	2338	2120	2259	2168	1752	1663	1782	1380
BC	1A5a	89	97	125	91	101	101	98	90	80	79	95	79	88	76	76	71	81	78	53	96	86	100	113

HM (Unit = g)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022
Pb	1A1a	7541108	6165047	3991076	4221131	3633488	2266111	2549808	2655085	2319559	1914728	2062325	2236269	2101319	3263587	2656844	2121464	2378973	2312662	2648614	2144187	2581283	2553799	2599213	2439894	2115641	2106953	2036387	2024422	2188937	1962530	1684322	1679446	1800381
Pb	1A2d	6199193	6184953	5377439	5115145	5750233	5305557	4914043	5386076	5348231	5478129	5049884	4567465	5860238	4170206	5104381	5061309	5659092	4663096	4079854	2640362	3414964	3382142	3411724	3382506	3708921	3501368	3533008	4021165	5140476	2943639	2563645	2880887	1842554
Pb	1A2f	2873152	1998141	2325899	2002794	2071174	2362165	2398164	2748927	2899119	2990336	3045669	3098517	3231079	3018616	3070723	3153785	3149247	3122309	3201364	1671292	2254755	2333420	1846126	1895146	1735202	1539310	1688250	1763165	922537	711870	667047	686440	646251
Pb	1A3bi	166003032	140003030	94003029	37002853	422922	2884	2785	2863	2825	2810	2714	2758	2817	2847	2907	2907	2896	2911	2804	2771	2727	2655	2609	2573	2549	2520	2509	2479	2462	2420	2246	2272	2119
Pb	1A3bvi	7220217	7047612	7005224	6946638	6932268	7021807	7071452	7219182	7384006	6575157	5632311	4655604	3664333	2647258	1584931	494393	498318	483049	480981	474675	478776	479305	474797	479973	486245	486814	491181	486694	488342	485007	465634	467420	460936
Pb	1A4bi	861950	716400	826750	702600	1051250	546100	575250	565950	575750	553450	518150	577250	567400	576320	581620	606770	584920	603720	576395	603545	670875	564790	612230	572740	576370	543720	585950	568610	558500	546695	499480	559870	512225
Pb	1A5a	261944	346435	143807	173344	140944	189655	217611	203194	215465	457809	216736	288930	493404	413998	507150	508493	415358	357663	435650	502691	548346	599974	663993	575603	637734	621932	757607	758404	494619	1069348	815222	1334681	1653001
Pb	2C1	34463226	16209473	30744363	32831303	40613400	47814170	23703730	5433394	10142714	8211759	7974043	7581211	7675760	4552150	5523760	2503460	5386030	2675060	1278880	2103340	3916490	2616730	400090	271820	494780	261730	331550	364510	376403	395152	517680	504186	424990
Pb	2C7c	80081000	45130700	9048000	6158200	3140600	566800	1970800	3957900	2418532	1066244	342322	797806	643630	318300	1048350	892790	718800	632730	349290	404360	424090	624720	341980	464620	783180	444690	476970	422748	298060	262960	276474	376115	288060
Pb	2G	310273	355575	736359	815431	1349291	1111409	634236	1018465	892001	1766707	1073962	1111823	1399112	1197770	1353671	1457545	1700462	1969688	1827946	1227780	1334072	1110914	1452870	1066049	1155724	1173281	1181068	1021338	1113300	890581	365405	629620	1061220
Cd	1A4bi	132905	131228	134123	131702	144843	120846	129781	130145	134793	131257	122739	140105	140976	144775	146847	154946	148319	155126	153614	161926	179883	153863	167949	158026	159956	150852	164040	160576	157776	155039	142500	159801	146855
Cd	2A3	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	180000	240000	140000	160000	260010	160010	31429
Cd	2C1	390235	222028	521680	666126	899140	997940	499700	51778	104558	63562	124535	127149	125420	60360	93400	98600	121250	42160	24890	62350	150340	132440	22170	19590	18810	21640	8500	5456	5619	4034	4067	5889	6460
Cd	2C6	850040	850026	750003	760004	39004	70004	120001	102000	110000	150000	93000	87180	56860	63380	100100	104000	107000	105300	77500	46400	53600	63000	23540	20300	22700	24240	13630	13260	12000	10800	9600	9500	9810
Cd	2C7c	4203000	1601450	1000000	900100	600000	20000	229100	326150	425420	269230	63481	400510	101500	111630	251910	141490	71000	50050	61920	57780	60990	55010	36090	13470	4400	1880	15030	10105	6550	1810	1346	37326	38020
Cd	NATIONALTOTAL	6685517	3810991	3326608	3387145	2719917	2127088	1910398	1589909	1694208	1534708	1411567	1745355	1374855	1327504	1615304	1451257	1426369	1266394	1206362	1153573	1283189	1218950	1169833	1079546	919334	889455	939843	954889	881086	789051	695996	802762	779146
Cd	NTCOMPL(NECD)	6685517	3810991	3326608	3387145	2719917	2127088	1910398	1589909	1694208	1534708	1411567	1745355	1374855	1327504	1615304	1451257	1426369	1266394	1206362	1153573	1283189	1218950	1169833	1079546	919334	889455	939843	954889	881086	789051	695996	802762	779146
Cd	NTCOMPLIANCE	6685517	3810991	3326608	3387145	2719917	2127088	1910398	1589909	1694208	1534708	1411567	1745355	1374855	1327504	1615304	1451257	1426369	1266394	1206362	1153573	1283189	1218950	1169833	1079546	919334	889455	939843	954889	881086	789051	695996	802762	779146
Hg	1A1a	238577	188988	248310	312652	381049	294753	355679	317038	248400	220551	182082	225396	233026	291414	199556	180955	212189	207150	192473	190643	230586	185058	208577	211814	182574	167152	144547	146322	160000	152628	105260	135283	140402
Hg	1A2f	16961	16914	28184	24341	21770	33200	20204	13352	23674	14186	17288	16222	18338	15750	45512	34062	70201	25982	22529	35385	44743	25541	28026	21876	21195	23075	19489	26929	53299	33883	25326	15921	22803
Hg	1A4bi	23759	22814	23027	22838	25182	21160	22727	22738	23527	22888	21383	24377	24529	25179	25503	26832	25727	26858	26215	27577	30646	26100	28435	26717	27012	25477	27683	27087	26619	26170	24050	26986	24774
Hg	2C1	5000	3900	4000	5000	6000	6000	5000	16000	68700	40000	43120	57960	41540	147090	163340	345500	409320	329010	297630	245920	303130	254620	207520	159020	167020	121320	118120	91340	101750	131460	131250	94350	84520
Hg	2C6						70000	70000	100000	10000	10000	900	500	270	2500	3200	5500	5000	7000	6600	6460	2430	2910	1150	1280	1850	860	940	700	1480	1900	5200	6230	2880
Hg	2C7a	6500	6500	6500	6500	6500	6500	6500	6500	6500	6500	6500	6500	10	26700	10	10	9	8	7	5	6	5	3	3	3	3	3	4	4	4	3	4	4
Hg	2C7c	28000	70000	70000	15000	10000	1000	14000	4106	3886	700	600	1400	1800	1260	700	1000	800	800	230	210	720	140	760	400	490	800	290	7860	78320	6220	3220	4503	3503
Hg	NATIONALTOTAL	1086517	929912	891298	765522	808290	800803	865263	813375	692610	635768	603450	684586	672095	819134	753585	891503	1034604	873178	820859	756048	887526	755133	744774	761779	707004	621298	590721	581904	679302	586740	537080	518556	504918
Hg	NTCOMPL(NECD)	1086517	929912	891298	765522	808290	800803	865263	813375	692610	635768	603450	684586	672095	819134	753585	891503	1034604	873178	820859	756048	887526	755133	744774	761779	707004	621298	590721	581904	679302	586740	537080	518556	504918
Hg	NTCOMPLIANCE	1086517	929912	891298	765522	808290	800803	865263	813375	692610	635768	603450	684586	672095	819134	753585	891503	1034604	873178	820859	756048	887526	755133	744774	761779	707004	621298	590721	581904	679302	586740	537080	518556	504918

POP (Unit = mg)

		1990	1991	1992	1993	1994	1995	1996	1997	1998	1999	2000	2001	2002	2003	2004	2005	2006	2007	2008	2009	2010	2011	2012	2013	2014	2015	2016	2017	2018	2019	2020	2021	2022
DIOX	1A2d	1032	824	840	948	1020	1064	1107	1242	1312	1330	1386	1272	1107	1092	1111	912	1038	963	971	1107	1135	1174	1152	1459	2006	1550	1721	906	1018	879	804	797	664
DIOX	1A2gviii	399	1758	530	297	219	274	221	320	270	255	923	281	273	231	241	211	390	236	236	233	218	223	322	730	632	825	618	537	731	191	214	590	148
DIOX	1A4bi	900	904	903	908	944	850	914	918	952	928	868	991	999	1026	1041	1096	1049	1096	1083	1142	1268	1084	1182	1112	1125	1061	1154	1129	1109	1090	1002	1123	1031
DIOX	2C1	4552	4098	4440	4586	4902	5060	3073	3224	3251	3258	3273	3242	3222	1318	1317	1328	901	891	841	391	2871	1011	1440	1300	1570	540	790	557	1196	979	721	632	509
DIOX	5E	3498	3514	3417	2316	1760	2054	2067	1935	2091	1914	2055	2272	2260	1993	2245	2398	2606	2614	2891	1809	1842	1693	1603	1561	1423	1350	1448	1404	1361	1370	1251	1317	1271
HCB	1A4bi	213705	213556	217339	214706	232529	198265	213069	213873	221676	215980	201980	230784	232392	238755	242255	255805	244755	256157	254379	268264	297993	255145	278624	262255	265540	250420	272421	266776	262122	257603	236814	265550	244100
HCB	2B10a	29000000	29000000	29000000	29000000	29000000	29000000	29000000	29000000	29000000	29000000	29000000	8190000	2480000	460000	16700000	23010000	26600000	30700000	10300000	20000000	1500000	18800000	1960000	10200000	13970000	8930000	52000000	25500000	23900000	15450000	13200000	15100000	21900000
PCB	1A4bi	2480791	2509430	2514873	2523166	2630946	2360828	2540876	2552863	2648901	2582832	2414617	2762792	2786723	2864642	2906574	3068926	2936264	3074087	3050788	3217190	3573886	3059915	3341513	3145101	3184715	3003373	3267889	3200306	3144589	3090731	2842094	3187326	2929722
PCB	1B1b	1753200	1695600	1792800	3146400	3319200	3312000	3276000	3164400	3283200	3240000	3276000	3272400	3283200	3222781	3253403	3217061	3131773	3114025	3097541	2665037	2979680	3068644	3169840	3159367	3196022	3152225	3176172	3110648	3098560	3010406	2742401	3005881	2908919